So via the admin area you can normally edit orders that are not completed. On the order overview page you should see a button Edit. What this will do is cancel the old order and simply let you create a new order. Here you can change the quantity that has been ordered.
Best Answer
You can use the Quote repository
\Magento\Quote\Api\CartRepositoryInterface
At this case, you also need quote id also
DELETE a quote item from Quote
use
Magento\Quote\Model\Quote\Item\Repository
and use
deleteById($QuoteId, $itemId)
,method.