Wcf – How to host WCF through TCP ports

What's likely happening is that SignalData is indirectly changing the subscribers dictionary under the hood during the loop and leading to that message. You can verify this by changing

foreach(Subscriber s in subscribers.Values)

To

foreach(Subscriber s in subscribers.Values.ToList())

If I'm right, the problem will disappear.

Calling subscribers.Values.ToList() copies the values of subscribers.Values to a separate list at the start of the foreach. Nothing else has access to this list (it doesn't even have a variable name!), so nothing can modify it inside the loop.

You'll want something like this to increase the message size quotas, in the App.config or Web.config file:

<bindings>
    <basicHttpBinding>
        <binding name="basicHttp" allowCookies="true"
                 maxReceivedMessageSize="20000000" 
                 maxBufferSize="20000000"
                 maxBufferPoolSize="20000000">
            <readerQuotas maxDepth="32" 
                 maxArrayLength="200000000"
                 maxStringContentLength="200000000"/>
        </binding>
    </basicHttpBinding>
</bindings>

And use the binding name in your endpoint configuration e.g.

...
bindingConfiguration="basicHttp"
...

The justification for the values is simple, they are sufficiently large to accommodate most messages. You can tune that number to fit your needs. The low default value is basically there to prevent DOS type attacks. Making it 20000000 would allow for a distributed DOS attack to be effective, the default size of 64k would require a very large number of clients to overpower most servers these days.